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Table 4 Source groups identified for PM2.5 components and WQS estimated weights assigned for the source groups

From: Associations between long-term exposures to airborne PM2.5 components and mortality in Massachusetts: mixture analysis exploration

Sources

PM2.5 Components

All-cause

Cardiovascular Mortality

Respiratory Mortality

Weights estimated from WQS models on all 15 PM 2.5 components, sum the weights for identified source groups

G1: Heavy fuel oil combustion

V, Ni

0.0012

0.1369

0.0184

G2: Biomass burning

K

0.3682

0.2162

0.4065

G3: Crustal matter

Si, Ca

0.0099

0.1454

0.0045

G4: Non-tailpipe traffic source

Zn, Pb, Fe, Cu

0.4316

0.1012

0.1389

G5: Tailpipe traffic sourcea

EC, OC

0.0780

0.1286

0.1237

G6: Secondary particles, power plantsa

SO42−, NO3−, OC

0.1111

0.2717

0.3080

G7: Secondary particles, agriculture

NH4+

1.3×10− 8

3.2×10− 8

6.1×10− 9

G8: Unclear source

Br

8.8×10− 9

1.8×10− 9

1.8×10− 9

Weights estimated from WQS models on the identified source groups

G1: Heavy fuel oil combustion

V, Ni

1.4×10− 6

0.0021

0.0002

G2: Biomass burning

K

0.4073

0.2342

0.4511

G3: Crustal matter

Si, Ca

0.0006

0.1069

0.0010

G4: Non-tailpipe traffic source

Zn, Pb, Fe, Cu

0.4472

0.0792

0.1586

G5: Tailpipe traffic sourcea

EC, OC

0.1445

0.2678

0.2674

G6: Secondary particles, power plantsa

SO42−, NO3−, OC

0.0004

0.3096

0.1209

G7: Secondary particles, agriculture

NH4+

6.7×10− 6

0.0002

0.0006

G8: Unclear source

Br

6.9×10− 7

6.9×10− 10

0.0002

  1. Abbreviations: All-cause for all non-accidental mortality, Cardiovascular Mortality for cardiovascular diseases related mortality; Respiratory Mortality for respiratory diseases related mortality
  2. aWe have made an arbitrary split of OC between tailpipe traffic source and secondary particles (power plants): for the sums of the weights, 50% of the OC weights were summed into tailpipe traffic source, and the other 50% were summed into secondary particles (power plants) source; for the WQS models on source groups, 50% of the OC mass were summed into tailpipe traffic source, and the other 50% were summed into secondary particles (power plants) source